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The series generated another band which released two albums that received gold certification in Argentina.Lopilato was the face of the underwear brand Promesse from 2006-10.Having completed the recordings of Alguien Que Me Quiera, Lopilato accompanied Bublé on his Crazy in Love tour.In 2011, Lopilato made her first film outside Argentina, the Spanish thriller Predeterminados (directed by Jordi Arencón), as "Vera". Previously, she was in a relationship with Felipe Colombo in 2002.After being in a relationship for several years they broke up in 2005 and she started dating Mariano Martinez in 2005.
Lopilato joined the cast of the El Trece series Lobo as a villainess, opposite Ana Linares's character (Vanesa González).
In November 2010, FHM in Spain ranked her 17th on its annual list Las 100 mujeres más sexys del mundo.
In late 2010, Lopilato announced that she was planning to marry the Canadian singer Michael Bublé in April 2011.
She was nominated for a Martin Fierro Award as Best Supporting Actress in a drama.
In 2014, Lopilato starred in the comedy film Las Insoladas, directed by Gustavo Taretto (known for his previous film Medianeras).